Abstract
X-ray thermal diffuse scattering intensity patterns from phonons in a fcc δ-Pu–Ga alloy have been recorded using an 18 keV undulator x-ray beam with a beam diameter of 25 μm. The results are consistent with patterns calculated using the Born–von Karman force constant model of lattice dynamics, and support the pronounced softening of the transverse acoustic branch along the [111] direction observed from inelastic x-ray scattering measurements. This work demonstrates the feasibility of using a “large-grain, small beam” approach to study lattice properties, such as phonon dispersion curves, of materials not readily available in the form of large single crystals.
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