Abstract
We report high-resolution infrared Zeeman spectra in the region of transitions between electronic singlets of the ground 5I8 and the first excited 5I7 crystal-field manifolds of Ho3+ in 7LiYF4 in a magnetic field directed along the tetragonal c axis of the crystal. Well-resolved hyperfine structure exhibiting non-linear Zeeman hyperfine splittings and crossings of components is observed. The experimental data are successfully explained on the basis of crystal-field calculations.
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