Abstract
In the PUREX process, the first U-Pu purification cycle (1CUPu) is not efficient enough for the decontamination of uranium flow out of neptunium. In this context, molecules known for their strong complexing power for actinides(IV) in aqueous phase, such as acetohydroxamic acid (AHA) have been tested in batch experiments to strip Np and Pu from TBP solvent loaded with U. A phenomenological model was developed and with the help of this model, a flowsheet of a counter-current alpha barrier process was designed and tested in C17 glove boxes in ATALANTE facility. A decontamination factor DFU/Np of 480 was obtained, higher than DFU/Np required by UNIREP standards.
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