Abstract

For a circularly polarized single-color field at a central frequency of $2\omega$ the final electron momentum distribution upon strong field ionization does not carry any information about the phase of the initial momentum distribution. Adding a weak, co-rotating, circularly polarized field at a central frequency of $\omega$ gives rise to a sub-cycle interference pattern (holographic angular streaking of electrons (HASE)). This interference pattern allows for the retrieval of the derivative of the phase of the initial momentum distribution after tunneling $\phi^{\prime}_{\mathrm{off}}(p_i)$. A trajectory-based semi-classical model (HASE model) is introduced which links the experimentally accessible quantities to $\phi^{\prime}_{\mathrm{off}}(p_i)$. It is shown that a change in $\phi^{\prime}_{\mathrm{off}}$ is equivalent to a displacement in position space $\Delta x$ of the initial wave packet after tunneling. This offset in position space allows for an intuitive interpretation of the Wigner time delay $\Delta \tau_W$ in strong field ionization for circularly polarized single-color fields. The influence of Coulomb interaction after tunneling is investigated quantitatively.

Highlights

  • The appearance of a comb of discrete peaks in the energy distributions of electrons upon strong field ionization [1] of single atoms or molecules is well-known as above threshold ionization (ATI) [2,3,4]

  • Building on the simplified HASE model, it is shown that the angular distribution of main ATI peaks and sidebands can be used to infer the derivative of the phase of the initial momentum distribution, φoff, from experimentally accessible quantities

  • It is found that φoff can be related to changes of the Wigner time delay τW within the HASE model

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Summary

INTRODUCTION

The appearance of a comb of discrete peaks in the energy distributions of electrons upon strong field ionization [1] of single atoms or molecules is well-known as above threshold ionization (ATI) [2,3,4]. That have the same helicity are referred to as corotating twocolor (CoRTC) fields [see Fig. 1(a) for an example] In this case, the intensity of these rings in the electron momentum distribution is modulated as a function of the angle in the plane of polarization [8]. The intensity of these rings in the electron momentum distribution is modulated as a function of the angle in the plane of polarization [8] The abbreviation a.u. is used to indicate atomic units throughout the paper

THEORETICAL MODEL
NUMERICAL EXAMPLES WITHOUT OFFSET PHASE
NUMERICAL EXAMPLES WITH OFFSET PHASE
HASE AND OFFSETS OF THE BOUND WAVE FUNCTION IN POSITION SPACE
HASE AND THE WIGNER TIME DELAY
RECIPE FOR THE EXPERIMENTAL ACCESS TO
VIII. THE INFLUENCE OF COULOMB INTERACTION AFTER TUNNELING
Findings
CONCLUSION
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