Abstract

A techno-economic analysis was completed to compare the use of Hollow Fiber Membrane Modules (HFMM) with the more conventional structured packing columns as the absorber in amine-based CO2capture systems for power plants. In order to simulate the operation of industrial scale HFMMsystems, a two-dimensional model was developed and validated based on results of a laboratory scale HFMM. After successful experiments and validation of the model, a pilot scaleHFMMwas constructed and simulated with the same model. The results of the simulations, from both sizes of HFMM, were used to assess the feasibility of further up-scaling to a HFMM system to capture the CO2from an 800 MWe power plant. The system requirements – membrane fiber length, total contact surface area, and module volume – were determined from simulations and used for an economic comparison with structured packing columns. Results showed that a significant cost reduction of at least 50% is required to make HFMM competitive with structured packing columns. Several factors for the design of industrial scale HFMMrequire further investigation, such as the optimal aspect ratio (module length/diameter), membrane lifetime, and casing material and shape, in addition to the need to reduce the overall cost. However,HFMMwere also shown to have the advantages of having a higher contact surface area per unit volume and modular scale-up, key factors for applications requiring limited footprints or flexibility in configuration.

Highlights

  • The need to reduce the amount of CO2 that is emitted into the atmosphere is an issue that is being addressed globally

  • Specifications of the flue gas conditions, solvent conditions, and Hollow Fiber Membrane Modules (HFMM) designs for the two cases considered: with and without a direct contact cooler

  • Based on data from two experimental systems – a laboratory scale and a pilot scale – two membrane mass transfer coefficients resulted from the fit of the simulation results and the experimental data – the “ideal case” km and the “worse case” km’, respectively

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Summary

PART 2

989 > Post-Combustion CO2 Capture by Vacuum Swing Adsorption Using Zeolites – a Feasibility. 1035 > Hollow Fiber Membrane Contactors for Post-Combustion CO2 Capture: A Scale-Up Study from Laboratory to Pilot Plant Captage postcombustion du CO2 par des contacteurs membranaires de fibres creuses : de l’échelle laboratoire à l’échelle pilote industriel É. Erin Kimball1*, Adam Al-Azki, Adrien Gomez, Earl Goetheer, Nick Booth, Dick Adams and Daniel Ferre. Abstract — Hollow Fiber Membrane Contactors for CO2 Capture: Modeling and Up-Scaling to CO2 Capture for an 800 MWe Coal Power Station — A techno-economic analysis was completed to compare the use of Hollow Fiber Membrane Modules (HFMM) with the more conventional structured packing columns as the absorber in amine-based CO2 capture systems for power plants. Oil & Gas Science and Technology – Rev. IFP Energies nouvelles, Vol 69 (2014), No 6 and validated based on results of a laboratory scale HFMM. HFMM were shown to have the advantages of having a higher contact surface area per unit volume and modular scale-up, key factors for applications requiring limited footprints or flexibility in configuration

INTRODUCTION
EXPERIMENTAL
MODELING
Case Descriptions
Results for Module Requirements
Configuration Design Options
ECONOMIC COMPARISON WITH STRUCTURED PACKING COLUMNS
CONCLUSIONS
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