Abstract

A novel cross-linkable electron-transport material has been designed and synthesized for use in the fabrication of solution-processed OLEDs. The material exhibits a low LUMO level of -3.51 eV, a high electron mobility of 1.5×10-5 cm2 V-1 s-1 , and excellent stability. An average 9.3 % shrinkage in film thickness was observed for the film after thermal curing. A maximum external quantum efficiency (EQE) of 15.6 % (35.0 cd A-1 ) was achieved for blue-phosphorescent OLEDs by spin-coating and 13.8 % (31.0 cd A-1 ) for an ink-jet-printed device, both of which are better than the EQE of a control device prepared by vacuum-deposition (see figure).

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