High-fidelity multistate stimulated Raman adiabatic passage assisted by shortcut fields

Abstract

Multistate stimulated Raman adiabatic passage (STIRAP) is a process which allows for adiabatic population transfer between the two ends of a chainwise-connected quantum system. The process requires large temporal areas of the driving pulsed fields (pump and Stokes) in order to suppress the nonadiabatic couplings and thereby to make adiabatic evolution possible. To this end, in the present paper a variation of multistate STIRAP, which accelerates and improves the population transfer, is presented. In addition to the usual pump and Stokes fields it uses shortcut fields applied between the states, which form the dark state of the system. The shortcuts cancel the couplings between the dark state and the other adiabatic states thereby resulting (in the ideal case) in a unit transition probability between the two end states of the chain. Specific examples of five-state systems formed of the magnetic sublevels of the transitions between two degenerate levels with angular momenta $J_g=2$ and $J_e=1$ or $J_e=2$ are considered in detail, for which the shortcut fields are derived analytically. The proposed method is simpler than the usual "shortcuts to adiabaticity" recipe, which prescribes shortcut fields between all states of the system, while the present proposal uses shortcut fields between the sublevels forming the dark state only. The results are of potential interest in applications where high-fidelity quantum control is essential, e.g. quantum information, atom optics, formation of ultracold molecules, cavity QED, etc.