High-Q Tamm plasmon-like resonance in spherical Bragg microcavity resonators.

Abstract

This work proposes what we believe to be a novel Tamm plasmon-like resonance supporting structure consisting of an Au/SiO2 core-shell metal nanosphere structure surrounded by a TiO2/SiO2 spherical Bragg resonator (SBR). The cavity formed between the core metal particle and the SBR supports a localized mode similar to Tamm plasmons in planar dielectric multilayers. Theoretical simulations reveal a sharp absorption peak in the SBR bandgap region, associated with this mode, together with strong local field enhancement. We studied the modification of a dipolar electric emitter's radiative and non-radiative decay rates in this resonant structure, resulting in a quantum efficiency of ∼90% for a dipole at a distance of r=60n m from the Au nanosphere surface. A 30-layer metal-SBR Tamm plasmon-like resonant supporting structure results in a Q up to ∼103. The Tamm plasmon-like mode is affected by the Bragg wavelength and the number of layers of the SBR, and the thickness of the spacer cavity layer. These results will open a new avenue for generating high-Q Tamm plasmon-like modes for switches, optical logic computing devices, and nonlinear applications.