Abstract
Organic-inorganic hybrid perovskite CH3NH3PbI3 (MAPbI3) single crystals (SCs) have been widely investigated in photodetection and X-ray detection. However, external electric-field-driven ion migration seriously affect the stability of MAPbI3 SCs based optoelectronic devices. Self-powered device can operate without any external power supply, which is suitable for mitigating the ion migration of MAPbI3 SCs. To realize self-powered MAPbI3 SC based photodetector and X-ray detector, an asymmetric Au/CH3NH3PbI3 SC/Au planar Schottky structure is employed in this work. At 0 V, the self-powered photodetector can achieve the responsivity of 11.1 mA/W at the wavelength of 795 nm, and the sensitivity of the self-powered X-ray detector can reach 477.1 μC Gy-1cm-2 with the detection limit of as low as 140.3 nGy s-1. Moreover, the self-powered optoelectronic device exhibits good stability in both photodetection and X-ray detection. Most importantly, high-quality near-infrared bioimaging and X-ray imaging are successfully realized by the above self-powered optoelectronic device.
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