Abstract
A scheme of second and third harmonic generation from laser irradiated anharmonic carbon nanotubes (CNTs) embedded in silica is proposed. An intense ultra short laser pulse interacting with the array of CNTs displaces its electrons. When this displacement becomes comparable to the radius of electrons of CNTs, the restoring force of electrons varies nonlinearly with the displacement. As a result, plasmon resonance gets broadened and the large resonance absorption of the laser by the electrons of CNTs occurs. The power conversion efficiency of harmonic generation due to the anharmonicity of CNTs is much higher than that due to the ponderomotive force nonlinearity. The effect of amplitude modulated parameter on the amplitude of second and third harmonic is studied. The high amplitude of generated harmonics can be realized with the amplitude modulated laser as compared to ordinary unmodulated laser.
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