Abstract
A gas-flow circulation apparatus coupled with a TEA-CO2 laser has been developed for the purpose of the isotope separation experiments using a free electron laser (FEL). The working gaseous mixture filled in the reaction chamber was smoothly circulated by the ventilation fan. Using the reaction chamber with the large volume, the multi-photon dissociation of a SiF3I molecule was successfully demonstrated. The change of IR spectrum monitored on-line by a FT-IR spectrometer showed that the TEA-CO2 laser effectively assisted the multi-photon dissociation of the molecules by the FEL.
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