Abstract
HighlightsFreestanding multicapsular carbon fibers (MCFs) cloth was synthesized by electrospinning and applied as interfacial layer to regulate the plating/stripping behavior of Zn anodes.MCFs layer is supposed to uniformize the electric field and Zn2+ flux, and the moderate zincophilicity enables the bottom-up deposition of Zn on Zn@MCFs anode, thereby leading to high-quality and rapid Zn deposition kinetics.Superior electrochemical performance of Zn@MCFs is achieved in symmetrical, asymmetrical and Zn||MnO2 batteries, including long cycling life, high coulombic efficiency and excellent rate performance.
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