Abstract
The spin density distribution of itinerant electrons, neg, and their effect on pairwise correlations of localized spins S(t2g) of Mn4+ ions in cubic Sr1 − xLaxMnO3 antiferromagnet (x = 0.02, TN = 230 K, G type magnetic structure) is studied experimentally by nuclear magnetic resonance on 17O nuclei. The regions with neg > x, in which the local spin susceptibility of pairs of Mn atoms follows the dependence χ ∼ (T − Θ)−1 with Θ = 20(5) K, indicating the growth of ferromagnetic spin correlations of neighboring magnetic ions in these domains, are found in the paramagnetic phase. The fraction of Mn-O-Mn bonds (neg > x) increases with the decrease in the temperature. The interpenetrating meshes of Mn-O-Mn bonds with different densities of itinerant eg electrons form an antiferromagnetic metal phase below TN. The role of weak localization effects is discussed as the main origin of the magnetic inhomogeneity of the antiferromagnetic metal phase in Sr0.98La0.02MnO3.
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a callDisclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.
