Abstract

A fundamental understanding of the flow of polymer solutions through the pore spaces of porous media is relevant and significant to enhanced oil recovery and groundwater remediation. We present in this work an experimental study of the fluid rheological effects on non-Newtonian flows in a simple laboratory model of the real-world pores—a rectangular sudden contraction–expansion microchannel. We test four different polymer solutions with varying rheological properties, including xanthan gum (XG), polyvinylpyrrolidone (PVP), polyethylene oxide (PEO), and polyacrylamide (PAA). We compare their flows against that of pure water at the Reynolds () and Weissenburg () numbers that each span several orders of magnitude. We use particle streakline imaging to visualize the flow at the contraction–expansion region for a comprehensive investigation of both the sole and the combined effects of fluid shear thinning, elasticity and inertia. The observed flow regimes and vortex development in each of the tested fluids are summarized in the dimensionless and parameter spaces, respectively, where is the normalized vortex length. We find that fluid inertia draws symmetric vortices downstream at the expansion part of the microchannel. Fluid shear thinning causes symmetric vortices upstream at the contraction part. The effect of fluid elasticity is, however, complicated to analyze because of perhaps the strong impact of polymer chemistry such as rigidity and length. Interestingly, we find that the downstream vortices in the flow of Newtonian water, shear-thinning XG and elastic PVP solutions collapse into one curve in the space.

Highlights

  • Polymer solutions refer to aqueous solutions that contain dissolved high-molecular-weight polymers

  • Our current experimental results are in good agreement with the analysis presented in the paper as far as the range of Reynolds number and aspect ratio are concerned

  • We have experimentally investigated the fluid rheological effects on the flow of four different water-based polymer solutions, i.e., xanthan gum (XG), PVP, polyethylene oxide (PEO) and PAA, through a rectangular contraction–expansion microchannel

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Summary

Introduction

Polymer solutions refer to aqueous solutions that contain dissolved high-molecular-weight polymers. Polymer solutions have been increasingly used in the past decade to manipulate particles and cells in microfluidic devices for various chemical and biomedical applications [3,4,5,6] They are frequently used in enhanced oil recovery and groundwater remediation to improve the displacement of trapped oil from a reservoir rock [7] or contaminants from a subsurface aquifer [8]. These applications benefit from a comprehensive understanding of the flow of polymer solutions through the pore spaces of porous media [9,10]. The optical transparency of microfluidic devices fabricated in, for example, polydimethylsiloxane (PDMS) or poly(methyl methacrylate) (PMMA), enables pore-scale flow visualization using optical imaging [13,14,15]

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