Abstract

We present theoretical description of Voigt and Faraday effect based optically pumped magnetometers using the Floquet expansion. Our analysis describes the spin-operator dynamics of the first, $\hat{F}(t)$, and second, $\hat{F}^2(t)$, order moments and takes into account of different pumping profiles and decoherence effects. We find that the theoretical results are in good agreement with the experimental demonstrations over a wide range of fields and pumping conditions. Finally, the theoretical analysis presented here is generalized and can be extended to different magnetometry schemes with arbitrary pumping profiles and multiple radio-frequency fields.

Highlights

  • Atomic-vapor-based optically pumped magnetometers (OPMs) [1,2] have become state-of-the-art magnetic field sensors with numerous applications in very diverse areas, ranging from fundamental physics in searching for electric dipole moment (EDM) [3,4], to geophysical and space magnetometry, medicine, such as magnetoencephalography (MEG) [5,6] and magnetocardiography [7,8,9]

  • A number of d√ifferent OPM architectures have shown sensitivity of fT/ Hz, based on spin-exchange relaxation-free (SERF) magnetometers [10,11], radio-frequency excited spin with Mx and Mz magnetometers relying on a linear atomic response [12,13,14], and modulated light magnetometers producing nonlinear magneto-optical rotation (NMOR) [15,16] due to a nonlinear optical response of the atoms

  • Most of OPMs are based on a Faraday dispersive measurement, in which oriented states [see Fig. 1(a)] are prepared and probed by a detuned laser beam measuring the Faraday rotation induced by the spin-polarized sample

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Summary

INTRODUCTION

Atomic-vapor-based optically pumped magnetometers (OPMs) [1,2] have become state-of-the-art magnetic field sensors with numerous applications in very diverse areas, ranging from fundamental physics in searching for electric dipole moment (EDM) [3,4], to geophysical and space magnetometry, medicine, such as magnetoencephalography (MEG) [5,6] and magnetocardiography [7,8,9]. [19], in which an aligned state is prepared instead of an oriented one [see, for example, Fig. 1(b)] and read through paramagnetic resonance, i.e., nondispersive measurement This kind of state allows a vector magnetometer operation using radio-frequency fields [20] or, as it was proposed more recently [21], adopting an all-optical approach which performs a dual axis magnetometer based on the Hanle effect. [22] we have shown that it is possible to employ dispersive measurements based on Voigt rotation when working with aligned states driven by radio-frequency fields, showing vector magnetometry operation (see Fig. 2). We show that the general dynamics of the second moment in the Liouville space can be reduced to Bloch equations [see Eq (2)] and can be solved by employing the Floquet expansion This solution predicts sensitivity to all three vector components of the magnetic field as reported in the experimental work in [22].

DISPERSIVE OPTICAL MEASUREMENTS
Heisenberg-Langevin equations
Spin dynamics in the laboratory frame
Floquet expansion of the first moment in the laboratory frame
Dynamics of the second moments in the laboratory frame
Second moment matrix dynamics in the Liouville space
FLOQUET EXPANSION OF THE SECOND MOMENT OF THE SPIN OPERATOR
OPM response during the probe cycle
Second moment dynamics in the rotating frame
RESULTS
Second moments for aligned states
Optimization
VIII. CONCLUSIONS
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