Abstract
The flexible top-emitting white organic light-emitting diode (FTEWOLED) with a very high efficiency but a significant color alteration is achieved with a blue/red/blue sandwiched tri-emission-layer. The voltage-dependent recombination region alternation and the emission mechanism are systematically investigated through a delta-doping method and the time-resolved transient photoluminescence lifetime measurement. By locating the main exciton recombination region at the 4,4′,4″-Tris(carbazol-9-yl)-triphenylamine (TCTA) and 9,9-spirobifluoren-2-yl-diphenyl-phosphine oxide (SPPO1) interface, replacing the carrier-trapping red dopant guest with an orange guest that utilizes energy transfer mechanism, and using a P–I–N structure together with the FIrpic blue guest dopant to balance the electron and hole carriers, an extremely color stable and a very high efficient FTEWOLED is fabricated, with the resulting high current and power efficiencies of 22.7cd/A and 14.27lm/W, and a warm white illumination with a small chromaticity variation of (−0.0087, +0.0015) over a broad luminance range of more than four orders of magnitude. In addition, the performances can be further improved to 23,340cd/m2, 24.49cd/A and 15.39lm/W with a slight concentration alteration of the orange emitter.
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