Abstract

High-resolution small-spot resonant photoemission measurements of the Y 1− x U x Pd 3 alloy system have revealed the variation in the U 5f lineshape down to 1% uranium dilution. Qualitatively, the spectrum consists of a peak below E F and a second peak impinging on E F. As x decreases from 1 to 0, the first peak moves toward E F due to a process known as Fermi-level tuning. In addition, the relative intensity of the E F peak is observed to grow in accordance with the onset of Kondo-like transport properties.

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