Abstract

Abstract. Aerosols affect the atmosphere through direct interaction with short-wave and long-wave radiation and the microphysical properties of clouds. In this paper we report in detail on several mechanisms by which the short-term impact of dust on surface radiative fluxes can affect the dust loading of the atmosphere via modification of boundary-layer meteorology. This in turn affects the aerosol radiative forcing itself. Examples of these feedbacks between dust and boundary layer meteorology were observed during a series of dust storms in the Sahara and the eastern Mediterranean in April 2012. These case studies have been analysed using the Monitoring Atmospheric Composition and Climate – Interim Implementation (MACC-II) system. The radiative fluxes in the short-wave and long-wave spectra were both significantly affected by the prognostic aerosol–radiation interaction, which in turn impacted the meteorological simulation. Reduced incoming solar radiation below the aerosol layers led to a decrease in maximum surface temperatures and to a more stable thermal stratification of the lower atmosphere. This in turn forced weaker surface wind speeds and eventually smaller dust emissions. Moreover, we also observed a secondary impact of the aerosol radiative forcing, whereby horizontal gradients of surface temperature were increased at the edge of the dust plume, which led to local increases of surface wind speeds due to the thermal wind effect. The differentiated impact of the aerosol layer on surface pressure also contributed to the increase in surface wind speed and dust production in the same area. Enhanced long-wave radiative fluxes by the dust mass were associated with opposite processes. Less stable thermal stratification at night, brought mainly by higher minimum temperatures at the surface, caused stronger surface winds. At the edge of the dust storm, weaker horizontal temperature and pressure gradients forced lower winds and reduced dust production. Regarding dust emissions, short-wave radiative forcing had a larger impact than long-wave radiative forcing, corroborating several previous studies. For surface temperature, short-wave and long-wave contribution were close in intensity. These feedbacks were amplified when using data assimilation to build the aerosol analysis of the MACC-II global system. This led to an improvement in the short-term forecasts of thermal radiative fluxes and surface temperatures.

Highlights

  • 1.1 Aerosol impacts on meteorologyAerosol particles play an important role in the atmosphere through various mechanisms

  • This paper focuses on the dust episode of 18 April 2012 over the eastern Mediterranean but we include the analysis of another dust storm, which took place on 12 and 13 April 2012 in the central Sahara region, as more ground observations were available

  • The MACC-II global system was run with no dust aerosols, with the aerosol direct effect estimated from a climatology, i.e. in its pre-operational configuration, and with the aerosol direct effect estimated from prognostic aerosols

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Summary

Introduction

Aerosol particles play an important role in the atmosphere through various mechanisms They impact air quality and represent a serious public health issue, as shown by recent particulate matter (PM) pollution events in western Europe and China (Zhang et al, 2014; Sun et al, 2013). Aerosol particles influence the atmospheric radiative budget directly by scattering and absorbing short-wave and long-wave radiation The aerosol direct effect consists of the sum of two phenomena: scattering/absorption of incoming solar radiation and absorption/emission of long-wave radiation. The former reduces the amount of solar energy that reaches the surface and can cause a warming of the aerosol layer because of absorption. The radiative impact of aerosols is very dependent on their vertical distribution and surrounding environment: Choi and Chung (2014) showed that whether the aerosol layer is below or above a cloud layer will impact their radiative impact on the surface and on the atmosphere by an order of magnitude

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