Abstract

Neutron Resonance Transmission Analysis (NRTA) uses resonant absorption of neutrons to infer the absolute isotopic composition of a target object, enabling applications in a broad range of fields such as archeology, enrichment analysis of nuclear fuel, and arms control treaty verification. In the past, NRTA involved large user facilities and complex detector systems. However, recent advances in the intensity of compact neutron sources have made compact neutron imaging designs increasingly feasible. This work describes the Monte Carlo (MC) based design of a compact epithermal NRTA radiographic instrument, which uses a moderated, compact deuterium-tritium neutron source and an epithermal neutron detector. Such an instrument would have a wide range of applications and would be especially impactful for scenarios such as nuclear inspection and arms control verification exercises, where system complexity and mobility may be of critical importance. The MC simulations presented in this work demonstrate accurate time-of-flight reconstructions for transmitted neutron energies, capable of differentiating isotopic compositions of nuclear material with high levels of accuracy. A new generation of miniaturized and increasingly more intense neutron sources will allow this technique to achieve measurements with greater precision and speed, with significant impact on a variety of engineering and societal problems.

Highlights

  • Many high- and mid-Z nuclei exhibit neutron-induced resonances in the epithermal range

  • When combined with a shielded neutron detector, such a beam can constitute a novel instrument for isotope-specific radiography of objects composed of mid- and high-Z elements. In this Monte Carlo (MC)-based study, we focus on the optimization of compact DT-based platforms, showing the feasibility and practicality of such platforms when it comes to materials analysis

  • TOF energy reconstruction In all MC simulations, the distance from the surface of the moderator to the detector was set to 1.845 m as a balance between TOF reconstruction precision and geometrical efficiency

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Summary

Introduction

Many high- and mid-Z nuclei exhibit neutron-induced resonances in the epithermal range (from 1 eV to 100 eV). The transmitted spectrum exhibits attenuation dips at energies that uniquely map to the resonance energies of the nuclei in the target material. In these measurements, a pulsed neutron beam (e.g., via spallation by a proton beam) is used in combination with a detector sensitive to epithermal neutrons, such as a lithium doped scintillator or a boron doped microchannel plate (MCP).. In combination with known cross section data, the transmission spectrum can be used to precisely and simultaneously determine the identity and the areal density of the multiple isotopes that make up the target object. A pixelated detector can further provide two-dimensional coordinate information, which can be used to determine the two-dimensional areal density of the isotopes, producing isotopic imaging of the target

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