Fault reactivation in clay-rich rocks – effects of water-clay interactions

Abstract

Clay-rich rocks play an important role in critical practical applications, particularly as natural barriers in nuclear waste repositories and subsurface caprocks for CO2 storage. The interaction between electrostatically charged clay minerals and polar fluids (e.g., water) can lead to swelling or, under confined conditions, build-up of swelling stress. Fault closure by swelling in clay-rich rocks has been the focus of many studies. However, it remains unclear how water-clay interactions affect the stability of pre-existing faults, considering that in addition to changes in frictional properties, the stress state may also change due to the build-up of swelling stress. This study addressed this gap by conducting triaxial friction experiments on oblique saw-cut cylindrical samples. The upper half of the sample consisted of a clay-rich rock (Opalinus claystone) and the lower half of a permeable sandstone (Berea sandstone). The first set of experiments determined the friction slip envelope of the sandstone-claystone interface without fluid injection, at confining pressures ranging from 4 to 25 MPa, and a constant axial loading rate of 0.1 mm/min. These experiments showed a frictional strength well below Byerlee’s law, indicating that the Opalinus claystone dictates the strength of the two-material interface. Friction experiments with fluid injection were then performed at confining pressures of 10 and 25 MPa with a constant piston position (no axial loading) and an initial differential stress of about 70% of the expected yield stress. The aim was to compare the fluid pressures required to initiate slip in scenarios with and without fluid-clay interactions. For this, the experiments involved stepwise increases in fluid pressure through the injection of either deionized water (a polar fluid) or decan (a non-polar fluid). In one of the decane and one of the water injection experiments, fibre-optic strain sensors were attached to the sample surface. This allowed us to differentiate between poroelastic deformation within the matrix, deformation due to water-clay interaction, and elastic relaxation due to slip along the saw cut. The friction slip envelope based on decane injection experiments is within the uncertainty of the friction slip envelope based on the experiments with no fluid injection. In contrast, the water injection experiments indicate a weakening of the frictional interface. We interpret this weakening to be due to the transition of the claystone from a solid rock to a mud close to the saw-cut surface. This weakening was evident even at ambient fluid pressure, although the apparent stress state was below the yielding stress, indicating the need to consider swelling stress in initial water injection scenarios. In summary, our data suggest that water-clay interactions may reactivate pre-existing faults due to (1) the change of the frictional properties and (2) the build-up of swelling stress.