Abstract
High-resolution Fourier transform studies of the CO-stretching and CH 3-rocking bands of 13CH 3OH have been applied to the assignment of far-infrared (FIR) laser transitions optically pumped by CO 2 infrared (IR) lasers. The assignments are based on spectroscopic identification of the IR pump transitions at the reported offsets from the CO 2 laser lines and agreement between the FIR laser wavenumbers and values calculated from IR/FIR combination-loop relations. Wavenumbers are also predicted for further potential new FIR laser lines in transition systems that could be pumped by CO 2 and 13CO 2 cw and waveguide lasers.
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