Failure mechanisms and acoustic responses of cylindrical lithium-ion batteries under compression loadings

Abstract

To understand the crashworthiness safety of lithium-ion battery (LIB) comprehensively, acoustic emission (AE) testing technology is introduced to explore the mechanical response and failure mechanism. In this paper, the compression process and failure behavior of 18650 LIBs under plane compression, local indentation and three-point bending are experimentally investigated. The effects of indenter diameter, state of charge (SOC) and capacity of the battery on the force-voltage-temperature responses are discussed in detail. The relation between the failure behavior and acoustic response of LIB is studied in combination with AE detection technique. The results show that the deformation of the battery can be divided into three stages before the failure, including the stress on the shell, compression on the internal gap and electrolyte, and stress on the whole. The failure inside the battery is caused by fold, shear fracture, local buckling and tensile break under different loading forms. The smaller the diameter of the indenter is, the lower bearing capacity at the point of failure is. High-SOC batteries experience higher forces and displacements at the failure point. High-capacity batteries have poor bearing capacity and are more prone to thermal runaway. AE signal can be detected at special points during the compression. Combined with the acoustic response of the battery, the whole deformation process is divided into five stages. The researches will provide a guidance for the failure detection and safety evaluation of LIBs.