Abstract

Using a time-resolved detection scheme in scanning transmission X-ray microscopy (STXM), we measured element resolved ferromagnetic resonance (FMR) at microwave frequencies up to 10 GHz and a spatial resolution down to 20 nm at two different synchrotrons. We present different methods to separate the contribution of the background from the dynamic magnetic contrast based on the X-ray magnetic circular dichroism (XMCD) effect. The relative phase between the GHz microwave excitation and the X-ray pulses generated by the synchrotron, as well as the opening angle of the precession at FMR can be quantified. A detailed analysis for homogeneous and inhomogeneous magnetic excitations demonstrates that the dynamic contrast indeed behaves as the usual XMCD effect. The dynamic magnetic contrast in time-resolved STXM has the potential be a powerful tool to study the linear and nonlinear, magnetic excitations in magnetic micro- and nano-structures with unique spatial-temporal resolution in combination with element selectivity.

Highlights

  • In spintronics and magnonics, it is important to understand the magnetization dynamics on the micro- and nano-scale e.g., to be able to control the propagation of spin waves

  • These measurement techniques include but are not limited to: magneto optic Kerr effect (MOKE) [4], Brillouin light scattering (BLS) [5], magnetic force microscopy (MFM) [6], scanning thermal microscopy (SThM) [7], scanning electron microscopy with polarization analysis (SEMPA) [8], and X-ray photoemission electron microscopy (X-PEEM) [9]. For most of these measurement techniques, it is not possible to measure with element selectivity (MOKE, BLS, MFM, SThM and SEMPA), while other measurement techniques like X-PEEM can only probe the surface of the sample with element selectivity

  • We have shown a way to correctly separate the quantitative pure dynamic magnetic contrast from the background signal in scanning transmission X-ray microscope (STXM)-ferromagnetic resonance (FMR)

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Summary

Introduction

It is important to understand the magnetization dynamics on the micro- and nano-scale e.g., to be able to control the propagation of spin waves. Other measurement techniques have been combined with FMR excitation in order to measure a single nano-sized object in an ensemble These measurement techniques include but are not limited to: magneto optic Kerr effect (MOKE) [4], Brillouin light scattering (BLS) [5], magnetic force microscopy (MFM) [6], scanning thermal microscopy (SThM) [7], scanning electron microscopy with polarization analysis (SEMPA) [8], and X-ray photoemission electron microscopy (X-PEEM) [9]. It is possible to obtain quantitative information about the local precession angle in FMR and its relative phase within a given STXM-FMR experiment

Experimental Details
X-ray Absorption
XMCD Effect in STXM-FMR
Analysis of STXM-FMR Measurements
Raw Data Treatment
Precession Angle
Origin of the Background Signal
Experimental Verification of the Magnetic Nature of the Dynamic Contrast
Contrast Reversal with Helicity
Helicity versus Field Direction
Contrast Reversal for Spin Wave Excitations
Conclusions
Full Text
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