Abstract

We show that the coherence of an electron spin interacting with a bath of nuclear spins can exhibit a well-defined purely exponential decay for special (``narrowed'') bath initial conditions in the presence of a strong applied magnetic field. This is in contrast to the typical case, where spin-bath dynamics have been investigated in the non-Markovian limit, giving superexponential or power-law decay of correlation functions. We calculate the relevant decoherence time ${T}_{2}$ explicitly for free-induction decay and find a simple expression with dependence on bath polarization, magnetic field, shape of the electron wave function, dimensionality, total nuclear spin $I$, and isotopic concentration for experimentally relevant heteronuclear-spin systems.

Talk to us

Join us for a 30 min session where you can share your feedback and ask us any queries you have

Schedule a call

Disclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.