Abstract

DyCu (CsCl-type) orders antiferromagnetically at . By measuring magnetization curves, the (H, T) phase diagrams are established for magnetic fields applied along fourfold and threefold axes. On the basis of neutron diffraction experiments on single crystals, magnetic structures are associated with each of the phases seen. The spontaneous and field-stabilized structures are multiaxial, with moments pointing along threefold or twofold directions. The phase sequence in the ordered range of DyCu reveals antiferroquadrupolar couplings of trigonal symmetry.

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