Excitons in quantum dot molecules: Coulomb coupling, spin-orbit effects, and phonon-induced line broadening

Abstract

Excitonic states and the line shape of optical transitions in coupled quantum dots (quantum dot molecules) are studied theoretically. For a pair of electrically tunable, vertically aligned quantum dots we investigate the coupling between spatially direct and indirect excitons caused by different mechanisms such as tunnel coupling, Coulomb coupling, coupling due to the spin-orbit interaction, and coupling induced by a structural asymmetry. The peculiarities of the different types of couplings are reflected in the appearance of either crossings or avoided crossings between direct and indirect excitons, the latter ones being directly visible in the absorption spectrum. We analyze the influence of the phonon environment on the spectrum by calculating the line shape of the various optical transitions including contributions due to both pure dephasing and phonon-induced transitions between different exciton states. The linewidth enhancement due to phonon-induced transitions is particularly pronounced in the region of an anticrossing and it strongly depends on the energy splitting between the two exciton branches.