Abstract
AbstractThe behaviour of an element of the Raman scattering tensor is considered as the exciting frequency is tuned through the vibronic absorption spectrum of the scattering molecule. Certain observed features of Raman excitation profiles are explained, and some predictions made. Using some simplifying assumptions, we examine the limiting form of the scattering tensor in certain resonance situations. On the basis of symmetry considerations, we then outline expected variations in (and limits on) the depolarization ratio near resonance.
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