Abstract
For the reaction of He(23 S, 21 S) with CS2 we present a large body of experimental data: electron spectra, fluorescence spectra, electron-ion and electron-photon coincidence spectra. The combination of all these data allows us to characterize the reaction in great detail in a way which is rather direct and free of speculations. As for other molecules with positive electron affinity the charge exchanged channel He+ + CS 2 − plays an important role as intermediate state. It is possible to isolate experimentally the electron energy spectra which correspond to formation of the individual electronic CS 2 + states out of the intermediate He+ + CS 2 − state. This has not been achieved so far for CS2 or any other molecule by straightforward evaluation of experimental data.
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