Abstract

A new experimental method for unveiling the strong hyperfine interactions of multi-electron ion configurations is described. It consists in observing atomic spin precessions of nuclear-excited ions recoiling through vacuum in weak external transverse magnetic fields. Due to the strong hyperfine coupling the nuclear orientation follows the atomic precession, resulting in a rotation of the angular correlation of decayγ-rays. The method is illustrated using the long-lived 197keV19F (5/2+) state as probe. The observed large precessions as well as the strong attenuations of theγ-angular correlations are well accounted for by considering all possible configurations resulting from the coupling ofL-shell electrons in the relevant ionic charge states.

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