Abstract
In this paper, the absorption spectrum and the electron paramagnetic resonance spectra of the Cr 3+ ions in the KZnF 3 crystal are explained based on the complete energy matrix diagonalization procedure and a crystal-field-like model. The results agree well with the experimental data. It is also shown that the nearest neighbor F − ions deviate 1.429±0.0015° and −0.5122±0.0015° from their original position because of the K + vacancy.
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