Evidence of two-stage melting of Wigner solids

Abstract

Two-dimensional (2D) solid-liquid transition (SLT)~\cite{Mermin1966Absence,Mermin1968Crystalline,Kosterlitz1972Long} concerns fundamental concepts of long-range correlations vital to magnetism, superconductivity, superfluidity, and topological matters. A long sought-after example is the melting of a Wigner Crystal (WC)~\cite{Wigner1934Interaction} of electrons. Detection efforts have targeted distinctive collective modes such as pinning by disorder, resonant-frequency absorption of Goldstone modes, and melting transition. However, only one-step second-order melting of softly-pinned modes was reported. Without the evidence of genuine pinning as exhibited in the charge density waves (CDWs)~\cite{PinningCDW}, these modes are likely intermediate phases which are only part of a complete SLT. To verify if there is a WC-intermediate phase transition will not only provide a solid proof of a WC, but will also unveil the nature of the SLT in relation to the two-stage Kosterlitz-Thouless (KT) model~\cite{Kosterlitz1972Long,Kosterlitz1973Ordering,Halperin1978Theory,Nelson1979Dislocation,hexatic_ceperley,hexatic_nelson, Young1979Melting}. %(or dislocation pairs) above a critical temperature $T_c$. Through transport studies of ultra-dilute high-purity 2D systems, this work presents evidence for not only a WC, but also for a two-stage WC-liquid SLT mediated by a first-order WC-intermediate phase transition.