Abstract

Radioactivity concentrations of nuclides of the 232Th and 238U radioactive chains and 40K, 90Sr, 137Cs, and 239+240Pu were surveyed for raw and cooked food of the population in the Red River delta region, Vietnam, using α-, γ-spectrometry, and liquid scintillation counting techniques. The concentration of 40K in the cooked food was the highest compared to those of other radionuclides ranging from (23 ± 5) (rice) to (347 ± 50) Bq kg−1 dw (tofu). The 210Po concentration in the cooked food ranged from its limit of detection (LOD) of 5 mBq kg−1 dw (rice) to (4.0 ± 1.6) Bq kg−1 dw (marine bivalves). The concentrations of other nuclides of the 232Th and 238U chains in the food were low, ranging from LOD of 0.02 Bq kg−1 dw to (1.1 ± 0.3) Bq kg−1 dw. The activity concentrations of 90Sr, 137Cs, and 239+240Pu in the food were minor compared to that of the natural radionuclides. The average annual committed effective dose to adults in the study region was estimated and it ranged from 0.24 to 0.42 mSv a−1 with an average of 0.32 mSv a−1, out of which rice, leafy vegetable, and tofu contributed up to 16.2%, 24.4%, and 21.3%, respectively. The committed effective doses to adults due to ingestion of regular diet in the Red River delta region, Vietnam are within the range determined in other countries worldwide. This finding suggests that Vietnamese food is safe for human consumption with respect to radiation exposure.

Highlights

  • Natural radioactivity is caused by the presence of naturally occurring radioactive matter (NORM) in the Earth crust.Among others, potassium-40 (40K), uranium-238 (238U and its decay series), and thorium-232 (232Th and its decay series) represent the group of NORM radionuclides

  • The aim of this study was to survey for the concentrations of radionuclides in NORM and artificial radionuclides, of the 90Sr, 137Cs, and 239+240Pu in raw and ready-to-eat food, representing for the major diet of the Vietnamese population to elucidate the effluence of the processing method to the concentration of the radionuclides in food and to estimate the annual committed effective dose through ingestion

  • The activity concentration of 90Sr, 137Cs, and 239+240Pu in all the study food was lower than its limit of detection (LOD), respectively, of 50, 20, and 5 mBq kg−1 dw

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Summary

Introduction

Natural radioactivity is caused by the presence of naturally occurring radioactive matter (NORM) in the Earth crust.Among others, potassium-40 (40K), uranium-238 (238U and its decay series), and thorium-232 (232Th and its decay series) represent the group of NORM radionuclides. In addition to the NORM, several artificial radionuclides, e.g., strontium-90 (90Sr), cesium-137 (137Cs), and plutonium-239 +240 (239+240Pu), which were released due to the human activities during the late 1950s and early 1960s are still present in our environment (Vaca et al 2001; Cochran et al 1987). These natural and artificial radionuclides are long lived, the half-lives (T1/2) of 40K, 238U, 232Th, 239Pu/240Pu, 137Cs, and 90Sr are 1.3E9 a, 4.5E9 a, 1.4E10 a, 24E3/6.56E3 a, 33 a, and 28 a, respectively, and nowadays, these radionuclides are typically present in air, soil, and water in different levels of activity. Average radiation doses to various organs of the body represent an important pathway for long-term health considerations

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