Abstract
Electron paramagnetic resonance linewidth measurements as functions of orientation were made on single crystals of the eclipsed, layered series of compounds (NH 3(CH 2) n NH 3)CuCl 4, n = 2, 3, 4, for the temperature range 100 to 333 K. Static spin correlations and antisymmetric exchange contributions are sufficient to explain the orientationally dependent data of the linewidths of the n = 2 and n = 3 compounds of the series, but the n = 4 compound linewidth data require the addition of the secular part of the two-dimensional spin-diffusive effects.
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