Enhancing light emission near low-refractive-index contrast nanostructures via mirror-symmetry breaking

Abstract

A platform of recent interest and large application potential is one in which the light emitters are directly integrated with an optical metasurface. Plasmonic metals and high-refractive-index, dielectric Mie metasurfaces have been explored in this connection but have their challenges. We propose low-refractive-index, contrast nanostructured thin films for studying metasurface-emitter systems, specifically focusing on two configurations of practical importance: LED white light generation using color converting polymers and fluorescence-based sensing in aqueous media. To achieve light emission enhancement in a low-index contrast, low optical absorption setting, we exploit the excitation of quasi-bound states in the continuum modes in a mirror-symmetry broken grating. Our numerical study predicts widely tuneable sharp-linewidth emission enhancements, near-zero quenching, and large and controllable active volume in the grating vicinity, which are significant improvements in comparison with both plasmonic and high-index contrast, all-dielectric platforms. When compared with simple gratings, mirror-symmetry broken gratings give four times larger radiative enhancement. Our results are of interest in furthering experimental activity and realizing applications such as light converter for efficient white LEDs and smart detection electronics-integrated substrates for sensing.