Abstract
The (XRD) patterns of the samples Ni0.5Zn0.5Fe2O4 in the form of powder were prepared using the ball milling technique for 41, 67 and 90 hours and were annealed at 1073, 1273 and 1373 K and (Poly vinylidine Fluoride) (PVDF) and composite samples of x% Ni0.5Zn0.5Fe2O4/PVDF, (x% = 5, 10, 15, 20 and 25%) have been studied. The α phase decrease and β-phases increase by increasing the ferrite content suggesting less crystallinity producing an amorphous structure of PVDF at x = 25% ferrite where as β PVDF nucleates in the composites The electric polarization increases by increasing NZF content. The transition from ferromagnetic (order state) to paramagnetic (disorder state) occurs at Curie temperature TC (600K). The DC resistivity is nearly constant from 153k to 286k for all composite samples and then decreases at high temperature. The behavior of dielectric constant and dielectric loss was measured in the temperature range from 200K to 700K. With the increase of magnetic content, the saturation magnetization (Ms) value of the composites also increases.
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