Abstract

With the development of the microelectronics industry, there is a huge demand for flexible polymer dielectrics with excellent dielectric energy storage capacity, aimed at increasing dielectric constant and enhancing breakdown strength. In this study, the hydroxylated BiFeO3-loaded polyvinylidene fluoride(PVDF) composite films were prepared by electrostatic spinning techniques and the energy storage properties have been investigated. The results show that the dielectric constant and breakdown strength of the composites are effectively influenced by the hydroxylation modification and spatial structure. More interestingly, the seven-grade hydroxylated composite films exhibit a great enhancement of the excellent energy storage performances (Ue, ∼13.21 J/cm3; η, ∼66.2 %). This study demonstrates the immense potential of these composites as highly efficient dielectric materials suitable for use in energy storage capacitors.

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