Abstract
A pivotal step toward understanding unconventional superconductors would be to decipher how superconductivity emerges from the unusual normal state. In the cuprates, traces of superconducting pairing appear above the macroscopic transition temperature Tc, yet extensive investigation has led to disparate conclusions. The main difficulty has been to separate superconducting contributions from complex normal-state behaviour. Here we avoid this problem by measuring nonlinear conductivity, an observable that is zero in the normal state. We uncover for several representative cuprates that the nonlinear conductivity vanishes exponentially above Tc, both with temperature and magnetic field, and exhibits temperature-scaling characterized by a universal scale Ξ0. Attempts to model the response with standard Ginzburg-Landau theory are systematically unsuccessful. Instead, our findings are captured by a simple percolation model that also explains other properties of the cuprates. We thus resolve a long-standing conundrum by showing that the superconducting precursor in the cuprates is strongly affected by intrinsic inhomogeneity.
Highlights
A pivotal step toward understanding unconventional superconductors would be to decipher how superconductivity emerges from the unusual normal state
We report complementary linear conductivity measurements and take a fresh look at prior experimental results, to demonstrate that the emergence of superconductivity can be consistently explained with this minimal model
In any alternating-field experiment, magnetic and electric fields are related, and it is arbitrary if one designates the signal at frequency 3ω as proportional to nonlinear conductivity or susceptibility
Summary
A pivotal step toward understanding unconventional superconductors would be to decipher how superconductivity emerges from the unusual normal state. 37 and Methods), and a scaling of the data for different compounds with the characteristic scale Tc. Figure 1b shows our nonlinear conductivity data in dependence on the GL-reduced temperature ln(T/Tc) compared to a calculation of σ3 using anisotropic GL theory beyond mean field (see Methods), similar to ref.
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