Electromagnon excitations in modulated multiferroics

Abstract

The phenomenological theory of ferroelectricity in spiral magnets presented in [M. Mostovoy, Phys. Rev. Lett. 96, 067601 (2006)] is generalized to describe consistently states with both uniform and modulated-in-space ferroelectric polarizations. A key point in this description is the symmetric part of the magnetoelectric coupling since, although being irrelevant for the uniform component, it plays an essential role for the nonuniform part of the polarization. We illustrate this importance in generic examples of modulated magnetic systems: longitudinal and transverse spin-density wave states and planar cycloidal phase. We show that even in the cases with no uniform ferroelectricity induced, polarization correlation functions follow the soft magnetic behavior of the system due to the magnetoelectric effect. Our results can be easily generalized for more complicated types of magnetic ordering, and the applications may concern various natural and artificial systems in condensed matter physics (e.g., magnon properties could be extracted from dynamic dielectric response measurements).