Electrically driven cavity plasmons in Au nanowire over Au film

Abstract

Light emission via inelastic tunneling electrons is appealing for integrated optoelectronic devices due to its femtosecond time scale that can in principle allow terahertz modulation bandwidth. It has gained renewed interest since 2015 due to the improved quantum efficiency, highly tunable emission wavelength, linewidth, or directionality once the electrodes are designed as a plasmonic nanocavity. However, efficient construction of stable tunnel junctions with desired plasmonic resonances is still technically challenging because of the subnanometer precision required in the electrical and optical design. Here, we demonstrate an easily accessible electrically driven cavity plasmon in metal-insulator-metal (MIM) tunnel junctions, comprised by a Au nanowire (NW) across two separate ultrasmooth Au electrodes. Two layers of self-assembled thiol molecule defines a reliable tunneling barrier. The contribution from the localized cavity plasmons to the total light emission is found to be dominant over that from the propagating surface plasmon polariton in the MIM waveguide, different from the traditional explanations. This work introduces a simplified method for constructing electrically driven cavity plasmons using crystalline metals, which holds promise for applications in in situ chemical or biosensing and the development of flexible light-emitting metasurfaces.