Electrical properties and spin fluctuations studies of Y(Co 1− xNi x) 2 compounds

Abstract

Synthesis by arc melting, the structural and the electric properties of Y(Co 1− x Ni x ) 2 alloys were studied by X-ray diffraction (XRD) and four probe dc electrical measurements. XRD analysis (300 K) shows that all samples crystallize in a cubic MgCu 2-type structure. The lattice parameters linearly decrease with Ni content. Electrical resistivity for the Y(Co 1− x Ni x ) 2 intermetallic series was measured in a temperature range of 15–1100 K. The parameters involved in the dependence of resistivity on temperature were determined. Residual, phonon and spin fluctuations resistivity were separated from electrical resistivity using both the Matthiesen formula and the Bloch–Gruneisen formula. The spin fluctuations resistivity of the Y(Co 1− x Ni x ) 2 series are compared to the mean square amplitudes of spin fluctuations previously calculated by the Linear Muffin Tin Orbital-Tight Binding Approach method for these series in the literature. The contribution of spin fluctuations to total resistivity ρ sf is proportional to T 2 at low temperatures. The proportionality parameter strongly reduces across the Y(Co 1− x Ni x ) 2 series.