Abstract
Ground-state phase diagrams and magnetization curves of a spin-1 Heisenberg diamond cluster with two different coupling constants and uniaxial single-ion anisotropy are investigated in a presence of the external magnetic field with the help of exact diagonalization methods. It is shown that the spin-1 Heisenberg diamond cluster exhibits several remarkable quantum ground states, which are manifested in zero- and low-temperature magnetization curves as intermediate plateaus at one-quarter, one-half and three-quarters of the saturation magnetization. It is found that the width of the fractional magnetization plateaus depends basically on a relative strength of the coupling constants as well as uniaxial single-ion anisotropy, which may substantially shrink or even cause full breakdown of some intermediate magnetization plateaus. It is evidenced that a relatively weak uniaxial single-ion anisotropy of the easy-axis type considerably improves a theoretical fit of low-temperature magnetization curves of the tetranuclear nickel complex [Ni4 (μ-CO3)2(aetpy)8](ClO4)4 in a low-field region without spoiling the previous fit based on the fully isotropic Heisenberg model in a high-field region.
Submitted Version (
Free)
Published Version
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a call