Effect of temperature on the scintillation properties of pure LaCl3 and Cs2LiYCl6:Ce crystals for neutron spectroscopy

Abstract

The Lunar Vehicle Radiation Dosimeters (LVRAD) project, run by the Korea Astronomy and Space Science Institute, is currently in the detector R&D phase. Its mission is to measure the radiation exposure experienced by astronauts on the lunar surface and to search for water and radioactive isotopes. This study focuses on inorganic scintillator R&D for neutron spectroscopy, which is essential for the LVRAD project. Two candidates, pure LaCl3 and Cs2LiYCl6:Ce enriched with 95% 6Li (CLYC-6) detectors, were investigated in this work. Though their neutron spectroscopy performance meets radiation hardness requirements, the temperature-dependent performance of the detectors needs to be clearly understood to ensure reliable operation in space. Therefore, the performance of pure LaCl3 and CLYC-6 detectors was investigated for working temperatures ranging from -30∘C to +50∘C. The dimensions of the scintillators used for measurements were Φ1.5 inch × 1.0 inch for pure LaCl3 and Φ1.5 inch × 1.5 inches for CLYC-6. Scintillation performance was measured using a Hamamatsu H7195 photomultiplier tube with a 500 MHz flash analog-to-digital converter. The detectors were operated in a large temperature and humidity chamber across a temperature range from -30∘C to +50∘C, and the temperature dependence of the pulse shape discrimination performance for fast and thermal neutrons was measured using pure LaCl3 and CLYC-6, respectively. The effect of the temperature on the absolute light yield, energy resolution, and decay times was also measured. Based on the results, the pure LaCl3 and CLYC-6 detectors proved suitable for neutron spectroscopy for the LVRAD project.