Abstract
We investigated the effects of activated carbon, used as constructed wetlands (CWs) medium, on its ability to remove four emerging endocrine-disrupting chemicals (EDCs): bisphenol A (BPA), bisphenol F (BPF), bisphenol S (BPS) and 4-tert-butylphenol (4-tert-BP). Two types of CWs planted with common reed were constructed, one with pumice rock called normal CW and the other was amended with activated carbon (AC) called AC-CW. EDCs contaminated synthetic wastewater (5 mg/L of each) was treated by CWs for 8 weeks. AC-CW completely and sustainably removed all four EDCs (98–100%) starting immediately and continuing throughout the experiment. Removal performances of all EDCs by AC-CW were significantly higher than those by normal CW. After experiment, no BPA and BPF and very small amounts of BPS and 4-tert-BP were detected in AC. In AC-CW, final elimination step of EDCs might be biodegradation. In addition, bacterial populations on AC component of AC-CW were one–two orders higher than those on the pumice rock of normal CW. Therefore, in AC-CW, EDCs were initially adsorbed onto AC, where they could be effectively degraded by high bacterial population.
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