Abstract

In this study, we systematically document the link between dust episodes and local scale regional aerosol optical properties over Jaipur located in the vicinity of Thar Desert in the northwestern state of Rajasthan. The seasonal variation of AOT(500 nm) (aerosol optical thickness) shows high values (0.51 ± 0.18) during pre-monsoon (dust dominant) season while low values (0.36 ± 0.14) are exhibited during winter. The Ångström wavelength exponent has been found to exhibit low value (<0.25) indicating relative dominance of coarse-mode particles during pre-monsoon season. The AOT increased from 0.36 (Aprilmean) to 0.575 (May-June(mean)). Consequently, volume concentration range increases from April through May-June followed by a sharp decline in July during the first active phase of the monsoon. Significantly high dust storms were observed over Jaipur as indicated by high values of single scattering albedo (SSA(440 nm) = 0.89, SSA(675 nm) = 0.95, SSA870 nm = 0.97, SSA(1,020 nm) = 0.976) than the previously reported values over IGP region sites. The larger SSA values (more scattering aerosol), especially at longer wavelengths, is due to the abundant dust loading, and is attributed to the measurement site's proximity to the Thar Desert. The mean and standard deviation in SSA and asymmetry parameter during pre-monsoon season over Jaipur is 0.938 ± 0.023 and 0.712 ± 0.017 at 675 nm wavelength, respectively. Back-trajectory air mass simulations suggest Thar Desert in northwestern India as the primary source of high aerosols dust loading over Jaipur region as well as contribution by long-range transport from the Arabian Peninsula and Middle East gulf regions, during pre-monsoon season.

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