Direct X-ray detection of the spin Hall effect in CuBi

Abstract

The spin Hall effect, and its inverse, are important spin-charge conversion mechanisms widely investigated due to their fundamental importance in the development of spintronics devices. Its measurement has been mostly related to electrical detection schemes involving an interface with another magnetic material and thus, a combination of the properties of both materials as well as the interface are measured. The large scattering of reported results from these methods for the same material and temperature call out for a more direct and interface-free approach. Optical detection schemes have been successfully used for the determination of SHE in semiconductor. However, this approach has proven challenging for metallic systems, due to their considerably shorter spin diffusion lengths. Only recently, optical measurements for Pt and W have been reported [1].Considering that magnetic circular dichroism (XMCD) has become a reference tool for precision measurements of small or diluted magnetic signals, We propose the use of XMCD-PEEM microscopy for direct, interface-free determination of SHE in metals. In particular, we report the observation of spin separation due to SHE in a single layer of Bi-doped Cu (Cu95Bi5), a material in which giant SHE has been already reported [2,3]. We have performed interface free x-ray spectroscopy measurements at the Cu L3,2 absorption edges while applying electrical current to the sample. The sign of spin accumulation depends on the direction of the current and the amplitude of the X-ray magnetic circular dichroism (XMCD) signal scales with the density current and have different sign when measuring in the L2 or L3 absorption edges, as expected for SHE. We have measured an induced magnetic moment of (2.7 ± 0.5) x 10-12μB A-1 cm2 per Cu atom averaged over the probing depth, which is of the same order as for Pt measured by magneto-optics. Our results constitute the proof of concept for the direct, interface free and element-selective measurement of the SHE in a single material by means of X-ray spectromicroscopy and highlight the potential of CuBi for spin-charge conversion applications [4].  (a) Visualization of the spin accumulation in a Cu95Bi5 electrode. (b) XMCD signal.