Abstract

Elemental type-II superconducting niobium is the material of choice for superconducting radiofrequency cavities used in modern particle accelerators, light sources, detectors, sensors, and quantum computing architecture. An essential challenge to increasing energy efficiency in rf applications is the power dissipation due to residual magnetic field that is trapped during the cool down process due to incomplete magnetic field expulsion. New SRF cavity processing recipes that use surface doping techniques have significantly increased their cryogenic efficiency. However, the performance of SRF Nb accelerators still shows vulnerability to a trapped magnetic field. In this manuscript, we report the observation of a direct link between flux trapping and incomplete flux expulsion with spatial variations in microstructure within the niobium. Fine-grain recrystallized microstructure with an average grain size of 10–50 µm leads to flux trapping even with a lack of dislocation structures in grain interiors. Larger grain sizes beyond 100–400 µm do not lead to preferential flux trapping, as observed directly by magneto-optical imaging. While local magnetic flux variations imaged by magneto-optics provide clarity on a microstructure level, bulk variations are also indicated by variations in pinning force curves with sequential heat treatment studies. The key results indicate that complete control of the niobium microstructure will help produce higher performance superconducting resonators with reduced rf losses1 related to the magnetic flux trapping.

Highlights

  • Variation in electronic mean free path due to interstitial contamination and the occurrence of a minimum in the Bardeen-Cooper-Schrieffer (BCS)resistance component of surface resistance for an optimal mean free p­ ath[22]

  • This cell structure is clearly visible in in-plane bright field (BF) image of transmission electron microscopy (TEM), Fig. 1(f)

  • Shear deformation is a characteristic of most common material processing operations and is very relevant for Superconducting radio frequency (SRF) Nb where the Nb sheets are fabricated by rolling and successive heat treatments to form polycrystalline ­material[30]

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Summary

Introduction

Variation in electronic mean free path due to interstitial contamination and the occurrence of a minimum in the Bardeen-Cooper-Schrieffer (BCS)resistance component of surface resistance for an optimal mean free p­ ath[22]. A multi-scale collective pinning mechanism is suggested for rf dissipation in SRF c­ avities[26], and a recent review indicates pinning possibilities could be related to dislocation ­structures[27]. In this manuscript, we address the issue of microstructure influenced flux trapping based on a systematic study of a deformed bi-crystal microstructure undergoing successive heat treatments. DC magnetization measurements are used to quantify the flux pinning force in the samples These results demonstrate that better engineering of the Nb microstructures could lead to reproducibly low flux trapping and provide improved routes for the production of high Q0 for SRF cavities for accelerator and other rf applications

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