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Abstract
Abstract The electric dipole moments of o-ClC6H4PCl2 1, C6H5PF4 2, o-ClC6H4PF4 3, C6H5P(O)F2 4, C6H5P(O)HF 5. C6H5P(O)H(OH) 6, and o-ClC6H4P(O)Cl2 7, were determined in dilute benzene solution at 25°C. The phosphoryl bond moment PO in compounds 4, 5, and 7 was estimated using simple bond-additivity calculations. The results obtained were 4.55D, 3.64D, and 5.52D for compounds 4, 5, and 7, respectively. Dipole moments for compounds 2 and 3 were also calculated theoretically using INDO MO techniques. The calculated values differed from the experimental values by about 12%.
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