Dielectric breakdown via emergent nonequilibrium steady states of the electric-field-driven Mott insulator

Abstract

In this work, we explore the possibility of emergent nonequilibrium steady states arising from the electric-field-driven Mott insulator via the Keldysh-Floquet dynamical mean field theory (DMFT), which can determine the fully-interacting, nonequilibrium steady-state Green's functions with the noninteracting counterparts as an input to the DMFT self-consistency loop. Unlike the retarded component, obtaining the lesser Green's function for the noninteracting system presents an important obstacle since the thermalization of the noninteracting system still requires a precise understanding of the dissipation mechanism. A crucial breakthrough in this work is that the noninteracting lesser Green's function can be determined in terms of the Wannier-Stark ladder (WSL) eigenstates, which are thermalized via the standard canonical ensemble according to the Markovian quantum master equation. As a result, it is shown that the intricate interplay between strong correlation and large electric field can generate a sequence of two dielectric breakdowns with the first induced by a coherent reconstruction of the mid-gap state within the Mott gap and the second by an incoherent tunneling through the biased Hubbard bands. It is predicted that the reconstructed mid-gap state generates its own emergent WSL structure with a reduced effective electric field. The two dielectric breakdowns are mediated by a reentrant insulating phase, which is characterized by the population inversion, causing instability toward inhomogeneous current density states at weak electron-impurity scattering.