Abstract

In China, the government and the cigarette industry yearly lose millions in sales and tax revenue because of imitation cigarettes. Usually, visual observation is not enough to identify counterfeiting. An auxiliary analytical method is needed for cigarette brands identification. To this end, we developed a portable, low-cost electronic nose (e-nose) system for brand recognition of cigarettes. A gas sampling device was designed to reduce the influence caused by humidity fluctuation and the volatile organic compounds (VOCs) in the environment. To ensure the uniformity of airflow distribution, the structure of the sensing chamber was optimized by computational fluid dynamics (CFD) simulations. The e-nose system is compact, portable, and lightweight with only 15 cm in side length and the cost of the whole device is less than $100. Results from the machine learning algorithm showed that there were significant differences between 5 kinds of cigarettes we tested. Random Forest (RF) has the best performance with accuracy of 91.67% and K Nearest Neighbor (KNN) has the accuracy of 86.98%, which indicated that the e-nose was able to discriminate samples. We believe this portable, cheap, reliable e-nose system could be used as an auxiliary screen technique for counterfeit cigarettes.

Highlights

  • Gas sensors based on semiconducting metal oxides (MOX) have been successfully used in the detection of various gases [1,2]

  • The most common MOX gas sensors have a sensitive layer made of tin oxide (SnO2 ) [3], tungsten oxide (WO3 ) [4], or zinc oxide (ZnO) [5]

  • Neighbors from two machine learning methods indicated that MOX sensors network is able to discriminate cigarette brands

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Summary

Introduction

Gas sensors based on semiconducting metal oxides (MOX) have been successfully used in the detection of various gases [1,2]. An e-nose system usually consists of: a sensor array including multiple sensors that react in some repeatable way when exposed to volatile substances released by analytes, a data acquisition (DAQ) system for measuring and collecting the responses of sensor array with a computer program which analysis results. This powerful tool has assisted many fields in food analysis [7,8], such as beer quality inspection [9,10], quality level identification of tea [11], characterization of juices [12], and differentiation of aromatic flowers [13]. E-nose can be applied to the monitoring of air quality [14,15,16,17,18,19] of gases emitted by the soil [20,21]

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