Abstract
Structure-directing hydrogen bonding, the molecular symmetry of the guest, and charge matching between host and guest are used to assemble four-ring units into sodalite-type cage assemblies with the imposition of the molecular symmetry of the template (guest) onto the final framework structure. Variable charge matching with PPZ+ or PPZ2+ (mono- and diprotonated piperazine, respectively) is shown to give interrupted and expanded sodalite-type zincophosphate structures (shown on the right).
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